Power is always expressed in WATTS and symbolized by the letter P
Voltage is always expressed in VOLTS and symbolized by the letter E or V
Current is always expressed in AMPERES and symbolized by the letter I
What is the relationship these P, E and I ?
Technician can sort out the power formula in any formation on the following order.
Watt, P = I x E or
Current, I = P ÷ R or
Voltage, E = P ÷ I
3x AAA batteries = 1.5V X 3 = 4.5V
You increased the voltage to the LED's, they will draw only as much amperage as they can handle, and the socket/board/chip set should already be "regulated" and have a set ohm resistance. The output of the LED's that you have is static, with the exception of when the batteries die(dimming). Since it's hooked up to a power source, they should stay the same intensity. The only way you're going to get safe increases in output is to increase the quantity of LED's.
My flashlight puts out 180 lumens with a full charge(one high power LED, vs your cluster of LED's), and it's $145 flashlight. While I support your DIY nature, I doubt it will be beneficial to your growing.